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Solution-Processable Copper(Ⅰ) Thiocyanate(CuSCN) as Hole Transport Layers for BiI_3 Solar Cells

Zhangwei He  Tinglei Zhao  Huanyu Ma  Zhanao Tan  
【摘要】:The solar cells have emerged as a series of star technologies in utilization of renewable energy.However,the issues raised by the short lifetime of the photovoltaics and toxic processing have severely limited their potential applications.In this work,we develop a two-step environmentally friendly solution deposition method to fabricate bismuth triiodide(BiI_3) solar cells.Using the technique,we harvest large size crystals and obtained uniform morphology of BiI_3 film.In addition,we demonstrate the use of solution-processable copper(I) thiocyanate(CuSCN) as hole transport layers in BiI_3 solar cells.The devices display an overall power conversion efficiency of 0.8% under AM 1.5 G illumination.This work provides new strategies for achieving high-efficiency BiI_3 solar cells.

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